Volume 14, No. 7, December 2014, Pages 1875-1882 PDF(1.74 MB)
Is Alaska Truly the Great Escape from Air Pollution? – Long Term Source Apportionment of Fine Particulate Matter in Fairbanks, Alaska
Yungang Wang1, Philip K. Hopke2
1 Environmental Energy Technologies Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA
2 Center for Air Resource Engineering and Science, Clarkson University, Potsdam, NY 13699, USA
- Seven sources were identified: soil, gasoline, sulfate, diesel, wood smoke, road salt, and nitrate.
- The contributions of diesel, wood smoke, and sulfate were doubled on violation days.
- Winter heating is the most important factor affecting the air quality in Fairbanks, Alaska.
- Additional source apportionment using other receptor models and tracers is needed.
Alaska is generally considered to be a place that is one of the last great escapes from air pollution. However, they have not spent a winter in Fairbanks or the nearby village of North Pole, where the daily average PM2.5 concentration was 170 µg/m3 in December 2012 according to the Alaska Department of Environmental Conservation (DEC) Air Monitoring Network. In this study, source apportionment using Positive Factorization Matrix (EPA PMF 5.0) has been conducted based on the 2005 to 2012 Fairbanks PM2.5 compositional data including elements, sulfate, nitrate, ammonia, elemental carbon (EC), and organic carbon (OC) from the U.S. Environmental Protection Agency speciation network. Seven sources were identified: soil, gasoline, sulfate, diesel, wood smoke, road salt, and nitrate. The average contributions to PM2.5 of these seven sources were 3.4%, 16.3%, 19.5%, 14.3%, 40.5%, 1.5%, and 4.5%, respectively. Wood smoke provided the highest contributions to PM2.5. Its contributions were the lowest in 2007 (3.5 µg/m3) and peaked in 2009 (5.7 µg/m3). The winter contributions of sulfate, nitrate, diesel, road salt, and wood smoke were all substantially higher compared to other seasons. Wood smoke is the only source with weekend’s contribution greater than the weekdays’ corresponding to the times when residential wood combustion is more likely to occur. The contributions of diesel, wood smoke, and sulfate were approximately doubled on violation days (daily average PM2.5 higher than 35 µg/m3) compared to all days. This finding indicates that winter heating is the most important factor affecting the air quality in Fairbanks. In the future, additional source apportionment using other receptor models and tracers will need to be conducted to confirm these results.
Air pollution; Fine particular matter; Source apportionment; Positive matrix factorization; Wood combustion; Alaska.